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Category:Malaysian pop singersOxygen-Mediated Electrodeposited Perovskite Film of a Metal-Organic Framework for Highly Stable Nanodiscs with Trap-Free Energy Level Energies.
Transition-metal oxides (TMOs) have attracted attention as electrolyte materials for high-capacity rechargeable batteries because of their high theoretical capacity. However, the stability and charge/discharge cycle life of TMO-based solid-state lithium/sodium batteries have been hindered by the dissolution of the TMOs. Here, we synthesized a TMO-based perovskite film formed in a tube-like shape with a continuous crystalline structure for the first time in a metal-organic framework (MOF). This MOF film consisted of three 1D zigzag tubes that were linked together in a three-dimensional structure with a large specific surface area and active pores. A novel strategy to produce oxygen-mediated electrodeposited perovskite film on the tube-shaped MOF film was investigated. The conductive tube-shaped MOF-based perovskite film could be electrodeposited by using a KClO4 aqueous solution, and this film retained its crystalline structure without dissolution even after electrolyte incorporation. In addition, the oxygen in the MOF tube was found to be essential for the formation of the electrolyte-conductive perovskite film. This technique can be applied to the development of an all-solid-state rechargeable lithium/sodium battery that is free from the stability and cycle life issues associated with soluble TMOs.Meta
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